论文标题
在整体上的范德华的连续体中,与自杂交结合状态的强烈互动
Strong light-matter interaction with self-hybridized bound states in the continuum in monolithic van der Waals metasurfaces
论文作者
论文摘要
连续体(BICS)中的光子绑定状态是与过渡金属二甲化元素(TMDC)相结合的杰出纳米光子平台,但到目前为止,主要用作全型递质元素,与邻近的TMDC层,与TMDC层相邻的TMDC层,与应变,模式,模式重叠和物质集成相关。在这项工作中,我们在实验上首次证明了不对称依赖性的BIC共振在2D阵列的单片跨面阵列中,仅由纳米结构化的大量TMDC WS $ _2 $与BIC模式呈现出锋利和剪裁的线路,理想增强轻度互动的理想。几何变化可以以散装WS $ _2 $中激子共振的BIC共振进行调整,从而揭示了具有反划入模式的强耦合方案和116 MEV的Rabi分裂。利用BIC概念对BIC概念提供的辐射损失通道的精确控制,可以通过元图的几何不对称参数来量身定制RABI分裂。至关重要的是,耦合强度本身可以受到控制,并且被证明与材料内部损失无关。我们的BIC驱动整体式跨表面平台可以很容易地合并其他TMDC或激子材料,以提供以前不可用的基本见解和用于极化应用程序的实用设备概念。
Photonic bound states in the continuum (BICs) are a standout nanophotonic platform for strong light-matter coupling with transition metal dichalcogenides (TMDCs), but have so far mostly been employed as all-dielectric metasurfaces with adjacent TMDC layers, incurring limitations related to strain, mode overlap, and material integration. In this work, we experimentally demonstrate for the first time asymmetry-dependent BIC resonances in 2D arrays of monolithic metasurfaces composed solely of the nanostructured bulk TMDC WS$_2$ with BIC modes exhibiting sharp and tailored linewidths, ideal for selectively enhancing light-matter interactions. Geometrical variation enables the tuning of the BIC resonances across the exciton resonance in bulk WS$_2$, revealing the strong-coupling regime with an anti-crossing pattern and a Rabi splitting of 116 meV. The precise control over the radiative loss channel provided by the BIC concept is harnessed to tailor the Rabi splitting via a geometrical asymmetry parameter of the metasurface. Crucially, the coupling strength itself can be controlled and is shown to be independent of material-intrinsic losses. Our BIC-driven monolithic metasurface platform can readily incorporate other TMDCs or excitonic materials to deliver previously unavailable fundamental insights and practical device concepts for polaritonic applications.