论文标题

稀土卤化物perovskites cseubr $ _3 $和cseucl $ _3 $

Antiferromagnetic Order in the Rare Earth Halide Perovskites CsEuBr$_3$ and CsEuCl$_3$

论文作者

Straus, Daniel B., Klimczuk, Tomasz, Xu, Xianghan, Cava, Robert J.

论文摘要

批量的CSEUBR $ _3 $和CSEUCL $ _3 $在实验中被证明是磁性半导体,在NEEL温度分别为2.0 K和1.0 K时,在抗fiferromagnet上订购抗fiferromagnetors。鉴于据报道,据报道,纳米颗粒和CSEUCL $ _3 $的薄膜在类似的温度下订购了铁磁,我们观察到CSEUBR中的防铁磁订单$ _3 $ _3 $和CSEUCL $ _3 $的观察 材料。我们的密度功能理论计算也支持了CSEUCL $ _3 $可以用作可切换磁性材料的结论。

Bulk CsEuBr$_3$ and CsEuCl$_3$ are experimentally shown to be magnetic semiconductors that order antiferromagnetically at Neel temperatures of 2.0 K and 1.0 K respectively. Given that nanoparticles and thin films of CsEuCl$_3$ have been reported to order ferromagnetically at a similar temperature, our observation of antiferromagnetic ordering in CsEuBr$_3$ and CsEuCl$_3$ expands the possible applications of halide perovskites to now include spintronic devices where both ferromagnetic and antiferromagnetic devices can be fabricated from a single material. The conclusion that CsEuCl$_3$ can be used as a switchable magnetic material is also supported by our density-functional theory calculations.

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