论文标题

金属纳米颗粒阵列中的异常吸收:量子点光电子的强大工具

Anomalous Absorption in Arrays of Metallic Nanoparticles: A Powerful Tool for Quantum Dot Optoelectronics

论文作者

Caillas, Augustin, Suffit, Stéphan, Filloux, Pascal, Lhuillier, Emmanuel, Degiron, Aloyse

论文摘要

高贵金属纳米颗粒的周期性阵列是光子学中的象征性纳米结构。这些年来,它们具有维持局部表面等离子体共振的能力,以证明各种被动和主动的功能,例如偶极培养基和LED中的发光增强,以及光电传统探测器中的较高措施。在这里,我们表明,与纳米颗粒之间的电感电流环相关的其他磁共振以及可与横向电波访问相关的,并在具有亚波长度周期的密集阵列的极限中出现。此外,它们与系统等离子体的相互作用导致电磁吸收(EIA)的频谱锐利类似物。我们使用这些元信息来诱导PBS纳米晶体的活性层发射,吸收,光影和极化特性中的变化和增强,这说明了EIA超出被动功能的潜力,而在文献中迄今已证明了EIA的潜力。

Periodic arrays of noble metal nanoparticles are emblematic nanostructures in photonics. Their ability to sustain localized surface plasmon resonances has been used throughout the years to demonstrate a variety of passive and active functionalities such as enhanced luminescence in dipolar media and LEDs as well as higher responsivities in photoconductive detectors. Here, we show that additional magnetic resonances, associated with inductive current loops between the nanoparticles and accessible with transverse electric waves, emerge in the limit of dense arrays with subwavelength periods. Moreover, their interplay with the plasmons of the system results in spectrally sharp analogues of electromagnetically induced absorption (EIA). We use these metasurfaces to induce changes and enhancements in the emission, absorption, photoconduction, and polarization properties of active layers of PbS nanocrystals, illustrating the potential of EIA beyond the passive functionalities demonstrated so far in literature.

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