论文标题
可调窄带激发型光学TAMM状态由无金属的全有机结构启用
Tunable narrowband Excitonic Optical Tamm States enabled by a metal-free all-organic structure
论文作者
论文摘要
光学TAMM状态(OT)是在两个高度反射结构之间的界面上发生的限制光学模式。但是,由于需要强烈的反射率,因此他们具有高度可加工和无金属的柔性材料的启动已被证明具有挑战性。本文中,我们开发了仅基于有机聚合物材料的第一个支持OT的结构,该结构基于非临界,可用且易于加工的伴侣 - 摩托式 - 摩托式 - 统治光子平台。制造的结构存在较大的面积,由窄带多层聚合物分布的布拉格反射器(DBR),然后是J聚集的分子iCeci-Tonic材料的薄膜,该材料可以在窄带范围内充当高度反射的表面。我们利用DBR和反射分子层的窄带光谱响应来通过改变多层的周期性来调整OTS谱带,从而为基于可轻质集成的激激体设备的OTS结构的织物打开了大门,并具有成本效益效率的设计。
Optical Tamm States (OTS) are confined optical modes that can occur at the interface between two highly reflective structures. However, due to the strong reflectance required, their implemen-tation with highly processable and metal-free flexible materials has proven challenging. Herein, we develop the first structure supporting OTS based only on organic polymeric materials, demon-strating a photonic platform based on non-critical, widely available, and easily processable mate-rials. The structures fabricated present large areas and consist of a narrowband multi-layered polymeric Distributed Bragg Reflector (DBR) followed by a thin film of J-aggregate molecular exci-tonic material that can act as a highly reflective surface within a narrowband range. We take ad-vantage of the narrowband spectral response of the DBR and of the reflective molecular layer to tune the OTS band by varying the periodicity of the multilayer, opening the door for the fabrica-tion of OTS structures based on lightweight integrable excitonic devices with cost-effective proce-dures.