学术文献库

In crystalline materials, electron-phonon coupling (EPC) is a ubiquitous many-body interaction that drives conventional Bardeen-Cooper-Schrieffer superconductivity. Recently, in a new kagome metal $\rm{CsV_3Sb_5}$, superconductivity that possibly intertwines with time-reversal and spatial symmetry-breaking orders is observed. Density functional theory calculations predicted weak EPC strength,$λ$, supporting an unconventional pairing mechanism in $\rm{CsV_3Sb_5}$. However, experimental determination of $λ$ is still missing, hindering a microscopic understanding of the intertwined ground state of $\rm{CsV_3Sb_5}$. Here, using 7-eV laser-based angle-resolved photoemission spectroscopy and Eliashberg function analysis, we determine an intermediate $λ$=0.45~0.6 at T=6 K for both Sb 5p and V 3d electronic bands, which can support a conventional superconducting transition temperature on the same magnitude of experimental value in $\rm{CsV_3Sb_5}$. Remarkably, the EPC on the V 3d-band enhances to $λ$~0.75 as the superconducting transition temperature elevated to 4.4 K in $\rm{Cs(V_{0.93}Nb_{0.07})_3Sb_5}$. Our results provide an important clue to understand the pairing mechanism in the Kagome superconductor $\rm{CsV_3Sb_5}$.