论文标题
通用的Wilson循环方法,用于非线性光 - 互动
Generalized Wilson Loop Method for Nonlinear Light-Matter Interaction
论文作者
论文摘要
传统上,通过第一原则的理论方法研究了非线性光 - 物质相互作用,作为超快光学的核心,大量光伏,非线性光电传感和成像以及有效的纠缠光子的产生。但是,这种间接方法通常会遭受带退化和光学零的差异以及汇合问题和高度计算成本的差异。在这里,以移位矢量和移位电流电量张量为例,我们提出了一种规范不变的通用方法,以通过表示广义的Wilson loop中的浆果浆果曲率,量子指标和移位矢量来有效,直接计算非线性光学响应。这种广义的威尔逊循环方法避免了上述繁琐的挑战,并可以轻松实施和有效的计算。更重要的是,Wilson循环表示基于量子几何张量和量子几何势,对非线性光学过程和响应进行了简洁的几何解释,并且可以很容易地应用于研究其他激发态响应。
Nonlinear light-matter interaction, as the core of ultrafast optics, bulk photovoltaics, nonlinear optical sensing and imaging, and efficient generation of entangled photons, has been traditionally studied by first-principles theoretical methods with the sum-over-states approach. However, this indirect method often suffers from the divergence at band degeneracy and optical zeros as well as convergence issues and high computation costs when summing over the states. Here, using shift vector and shift current conductivity tensor as an example, we present a gauge-invariant generalized approach for efficient and direct calculations of nonlinear optical responses by representing interband Berry curvature, quantum metric, and shift vector in a generalized Wilson loop. This generalized Wilson loop method avoids the above cumbersome challenges and allows for easy implementation and efficient calculations. More importantly, the Wilson loop representation provides a succinct geometric interpretation of nonlinear optical processes and responses based on quantum geometric tensors and quantum geometric potentials and can be readily applied to studying other excited-state responses.