论文标题
活性胶体分子在活性梯度中
Active Colloidal Molecules in Activity Gradients
论文作者
论文摘要
我们考虑一个在活性梯度中形成活性胶体二聚体的两个活性布朗颗粒的刚性组装。我们分析表明,根据两个粒子的相对取向,活性二聚体在高活性或低活性区域中累积,分别对应于趋化性和抗凝集性。某些活性二聚体表现出趋化性和抗血性行为,具体取决于活性的强度。我们粗粒的福克 - 普兰克方法产生了有效的潜力,我们用来构建非平衡相图根据二聚体根据其战术行为进行分类。此外,我们表明,对于某些二聚体,运动的持久性与方向盘在宏观设备中的效果相似。这项工作对于设计自主的主动胶体结构可能很有用,这些胶体结构根据当地活动梯度来调整其运动。
We consider a rigid assembly of two active Brownian particles, forming an active colloidal dimer, in a gradient of activity. We show analytically that depending on the relative orientation of the two particles the active dimer accumulates in regions of either high or low activity, corresponding to, respectively, chemotaxis and antichemotaxis. Certain active dimers show both chemotactic and antichemotactic behavior, depending on the strength of the activity. Our coarse-grained Fokker-Planck approach yields an effective potential, which we use to construct a nonequilibrium phase diagram that classifies the dimers according to their tactic behavior. Moreover, we show that for certain dimers a higher persistence of the motion is achieved similar to the effect of a steering wheel in macroscopic devices. This work could be useful for designing autonomous active colloidal structures which adjust their motion depending on the local activity gradients.