论文标题

范德华异质结构中间接激子的远程量子运输

Long-range quantum transport of indirect excitons in van der Waals heterostructure

论文作者

Fowler-Gerace, L. H., Zhou, Zhiwen, Szwed, E. A., Butov, L. V.

论文摘要

长期的空间间接激子(IX)的寿命,也称为Interlayer激子,使IX可能会繁殖。范德华(Van der Waals)异质结构由原子上薄层的过渡金属二核苷层(TMDS)组成,有机会实现具有高结合能的激子,并为实现激子量子量子现象和激子设备提供了材料平台。深入研究了TMD异质结构中IXS的传播。但是,尽管有长期的IX寿命,但比空间直接激子(DXS)长的数量级长,这是一种相对短的IX传播,其$ 1/e $ n o $衰减距离$ d_ {1/e} $ d_ {1/e} $在TMD杂质构造的研究中据报道多达几美元。 IX繁殖的短距离源自面内电势,该电位定位激子并抑制激子的运输。特别是,TMD异质结构中预测的显着平面内Moiré电位可能会导致IX传播的障碍。在这项工作中,我们在摩尔斯$ _2 $/WSE $ _2 $异质结构中意识到宏观上长距离IX传播,$ d_ {1/e} $到达$ \ sim \ sim 100 $ $ $μ$ m。 IX传播的强大增强是使用异质结构中DXS的光激发共鸣实现的。 IX传播的强大增强源于IX定位和散射的抑制,并且在量子状态下观察到。

Long lifetimes of spatially indirect excitons (IXs), also known as interlayer excitons, make possible long-range IX propagation. Van der Waals heterostructures composed of atomically thin layers of transition-metal dichalcogenides (TMDs) give an opportunity to realize excitons with high binding energies and provide a materials platform for the realization of both excitonic quantum phenomena and excitonic devices. Propagation of IXs in TMD heterostructures is intensively studied. However, in spite of long IX lifetimes, orders of magnitude longer than lifetimes of spatially direct excitons (DXs), a relatively short-range IX propagation with the $1/e$ decay distances $d_{1/e}$ up to few $μ$m was reported in the studies of TMD heterostructures. The short-range of IX propagation originates from in-plane potentials, which localize excitons and suppress exciton transport. In particular, significant in-plane moiré potentials predicted in TMD heterostructures can cause an obstacle for IX propagation. In this work, we realize in a MoSe$_2$/WSe$_2$ heterostructure a macroscopically long-range IX propagation with $d_{1/e}$ reaching $\sim 100$ $μ$m. The strong enhancement of IX propagation is realized using an optical excitation resonant to DXs in the heterostructure. The strong enhancement of IX propagation originates from the suppression of IX localization and scattering and is observed in the quantum regime.

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