论文标题
非线性介电元脉冲的谐振性手性效应
Resonant chiral effects in nonlinear dielectric metasurfaces
论文作者
论文摘要
我们研究了连续体(quasi-bics)中支持多极MIE共振和准结合状态的不对称硅元脉体中线性和非线性手流效应的谐振增强。我们在理论上证明并观察到准BIC共振处的明显线性圆形二色性。我们进一步发现,对于MIE共振和一些准BIC模式,局部场增强和第三谐波信号都很大。我们通过采用关键耦合的概念来解释非线性增强的选择性,这对中等较大的辐射质量因素($ q $ caxption)的模式更有利。我们展示了与第三次谐波一代高效率和大型非线性圆形二色性效率相关的实验性强非线性手势反应,从$+++0.918 \ pm0.049 $到$ -0.771 \ pm0.004 $,对于具有不同非对象的样品。我们相信我们的结果表明了在介电谐振元面积中进行工程非线性手势反应的一般策略。
We study the resonant enhancement of linear and nonlinear chiroptical effects in asymmetric silicon metasurfaces supporting multipolar Mie resonances and quasi-bound states in the continuum (quasi-BICs). We demonstrate theoretically and observe in experiment the pronounced linear circular dichroism at the quasi-BIC resonances. We further find that both local field enhancement and third-harmonic signal are large for Mie resonances and some quasi-BIC modes. We explain the selectivity of the nonlinear enhancement by employing the concept of critical coupling being more favorable for the modes with moderately large radiative quality factors ($Q$ factors). We demonstrate experimentally strong nonlinear chiroptical response associated with high efficiency of the third-harmonic generation and large nonlinear circular dichroism varying from $+0.918\pm0.049$ to $-0.771\pm0.004$ for the samples with different asymmetries. We believe our results suggest a general strategy for engineering nonlinear chiroptical response in dielectric resonant metasurfaces.