论文标题

使用光学涡流梁研究山谷松弛的稳态方法

A steady state approach for studying valley relaxation using optical vortex beam

论文作者

Pattanayak, Aswini Kumar, Das, Pritam, Dhara, Avijit, Chakrabarty, Devarshi, Paul, Shreya, Gurnani, Kamal, Brundavanam, Maruthi Manoj, Dhara, Sajal

论文摘要

单层过渡金属二分法中的自旋谷耦合产生了山谷极化和相干效应,受到了由激子 - phonon,Ickiton-Phonon引起的间隔散射的限制,激子IMBRINE和电子孔交换相互作用(EHEI)。我们通过使用高阶光学涡流束的光子分布来控制质量动量(COM)的激动子中心(COM)来探索一种调整EHEI的方法。因此,我们已经观察到激子依赖性山谷去极化和反矫正性,这使我们能够测量与稳态测量中与山谷动力学相关的时间表。我们探测山谷动力学的稳态技术可以打开一个新的范式,以探索二维系统中激子的物理。

Spin-valley coupling in monolayer transition metal dichalcogenides gives rise to valley polarization and coherence effect, limited by intervalley scattering caused by exciton-phonon, exciton-impurity, and electron-hole exchange interaction (EHEI). We explore an approach to tune the EHEI by controlling excitons center of mass momentum (COM) utilizing the photon distribution of higher-order optical vortex beam. By virtue of this, we have observed excitons COM-dependent valley depolarization and decoherence which gives us the ability to measure the timescale associated with valley dynamics in the steady-state measurement. Our steady-state technique to probe the valley dynamics can open up a new paradigm to explore the physics of excitons in two-dimensional systems.

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