论文标题
直接可视化和原子尺度缺陷对六角硼的光电特性的影响
Direct visualization and effects of atomic-scale defects on the optoelectronic properties of hexagonal boron nitride
论文作者
论文摘要
由于其许多非凡的特性,六角硼(HBN)在过去几年引起了很多关注。其中包括具有具有出色光学特性的单光子发射器的存在,这使其成为众多光子技术的理想候选者。然而,尽管实验结果和理论计算大量,但负责观察到的发射的缺陷的结构仍在争论中。在这项工作中,我们在环境条件下使用原子力显微镜可视化HBN中的单个原子尺度缺陷,并观察到来自光学稳定的发射器的多个狭窄的发射线。对缺陷的结构的直接观察结合了其带状结构和电子特性的密度功能理论计算,使我们能够将几个单光子过渡的存在与观察到的缺陷联系起来。我们的工作阐明了HBN中单光子发射的起源,这对于在光电和量子技术中高质量发射器的理解和可调性很重要。
Hexagonal boron nitride (hBN) is attracting a lot of attention in the last years, thanks to its many remarkable properties. These include the presence of single-photon emitters with superior optical properties, which make it an ideal candidate for a plethora of photonic technologies. However, despite the large number of experimental results and theoretical calculations, the structure of the defects responsible for the observed emission is still under debate. In this work, we visualize individual atomic-scale defects in hBN with atomic force microscopy under ambient conditions and observe multiple narrow emission lines from optically stable emitters. This direct observation of the structure of the defects combined with density functional theory calculations of their band structures and electronic properties allows us to associate the existence of several single-photon transitions to the observed defects. Our work sheds light on the origin of single-photon emission in hBN that is important for the understanding and tunability of high-quality emitters in optoelectronics and quantum technologies.