论文标题

几乎理想的简单轴三角量子量子反铁磁铁Na $ _2 $ baco(po $ _4 $)$ _ 2 $

Spin Supersolidity in Nearly Ideal Easy-axis Triangular Quantum Antiferromagnet Na$_2$BaCo(PO$_4$)$_2$

论文作者

Gao, Yuan, Fan, Yu-Chen, Li, Han, Yang, Fan, Zeng, Xu-Tao, Sheng, Xian-Lei, Zhong, Ruidan, Qi, Yang, Wan, Yuan, Li, Wei

论文摘要

原型模型及其物质化身是对量子磁性理解的基石。从理论上讲,我们在这里表明,最近合成的磁化合物na $ _2 $ baco(po $ _4 $)$ _ 2 $(NBCP)是$ s = 1/2 $ s = 1/2 $三角形静态的抗fiferromagnet的罕见,几乎是理想的材料实现,并具有大量的易于轴承旋转交换的旋转交换。通过将自动参数搜索和张量 - 网络模拟结合在一起,我们将其对该材料的微观模型描述与现实的模型参数相结合,该模型不仅可以很好地拟合实验性热力学数据,而且还可以在没有进一步调整参数的情况下重现测得的磁化曲线。根据已建立的模型,NBCP拥有一个自旋超olid状态,该状态既打破晶格翻译对称性和自旋旋转对称性。这样的状态是长期以来的超胚膜状态的自旋类似物,被认为存在于固体和光学晶格系统中,并具有相似的特征。因此,NBCP代表了一个理想的基于材料的平台,用于探索超偏度的物理及其量子和热熔化。

Prototypical models and their material incarnations are cornerstones to the understanding of quantum magnetism. Here we show theoretically that the recently synthesized magnetic compound Na$_2$BaCo(PO$_4$)$_2$ (NBCP) is a rare, nearly ideal material realization of the $S=1/2$ triangular-lattice antiferromagnet with significant easy-axis spin exchange anisotropy. By combining the automatic parameter searching and tensor-network simulations, we establish a microscopic model description of this material with realistic model parameters, which can not only fit well the experimental thermodynamic data but also reproduce the measured magnetization curves without further adjustment of parameters. According to the established model, the NBCP hosts a spin supersolid state that breaks both the lattice translation symmetry and the spin rotational symmetry. Such a state is a spin analogue of the long-sought supersolid state, thought to exist in solid Helium and optical lattice systems, and share similar traits. The NBCP therefore represents an ideal material-based platform to explore the physics of supersolidity as well as its quantum and thermal melting.

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