论文标题
铁电隧道连接处多域的动力学
Dynamics of Multi-Domains in Ferroelectric Tunnel Junction
论文作者
论文摘要
在铁电隧道连接(FTJ)中发现巨型隧道电气稳定(TER)铺平了一种未来派的可能性,它将FTJ用作具有极高的/OFF/OFF比例的Biscebable电阻器件。在过去的20年中,许多研究报告说,铁电材料中多域的形成是最大程度地减少总系统能量的过程。基于相位模拟的最新研究表明,域成核/运动基本上会显着改变铁电材料的静电。但是,域动力学对FTJ中量子运输的影响仍然难以捉摸。本文介绍了铁电隧道连接处多域动力学的全面研究。对本文的分析是双重的。首先,我们研究了域动力学对FTJ中静电的影响。随后,获得的静电学用于研究隧道电流的变化,而TER起源于多域动力学。我们表明,在铁电区域中开/关的电流密度和局部变化。此外,由于周期域纹理,该设备的静电和量子传输表现出振荡性。电流密度在铁电中显示出正弦/余弦的分布,并且观察到电流密度大约十年的局部变化。当前密度的这些局部波动会导致设备的开/OFF比率振荡。还讨论了实现统一和最大TER的优化技术。通过求解耦合的2D Poisson方程和Landau-Ginzburg方程来得出2D分析和显式模型。该模型通过最大程度地减少净铁电能(去极化+游离+梯度能量密度)来结合域的开关和成核。此外,还研究了底部绝缘体层对铁电梯度能量的影响。
The Discovery of giant tunnel electroresistance (TER) in Ferroelectric Tunnel Junction (FTJ) paves a futuristic possibility of utilizing the FTJ as a bistable resistive device with an enormously high ON/OFF ratio. In the last 20 years, numerous studies have reported that the formation of multidomain in ferroelectric material is an inevitable process to minimize the total system energy. Recent studies based on phase-field simulations have demonstrated that domain nucleation/motion substantially alters the electrostatics of a ferroelectric material. However, the impact of domain dynamics on quantum transport in FTJ remains elusive. This paper presents a comprehensive study of multidomain dynamics in a ferroelectric tunnel junction. Analysis of this article is twofold; firstly, we study the impact of domain dynamics on electrostatics in an FTJ. Subsequently, the obtained electrostatics is used to study the variations in tunneling current, and TER originated from multidomain dynamics. We show that ON/OFF current density and TER vary locally in the ferroelectric region. Furthermore, the device's electrostatics and quantum transport exhibit an oscillatory nature due to periodic domain texture. ON/OFF current density shows a sine/cosine distribution in ferroelectric, and approximately one-decade local variation in current density is observed. These local fluctuations in current density cause oscillations in the device's ON/OFF ratio. Optimization techniques to achieve a uniform and maximum TER are also discussed. A 2D analytical and explicit model is derived by solving coupled 2D Poisson's equation and Landau-Ginzburg equation. The model incorporates the switching and nucleation of domains by minimizing net ferroelectric energy (depolarization+free+gradient energy density). Furthermore, the impact of the bottom insulator layer on ferroelectric's gradient energy is also studied.