论文标题
液体结构有序在玻璃过渡,结晶和水的异常中的作用
Roles of liquid structural ordering in glass transition, crystallization, and water's anomalies
论文作者
论文摘要
液态是物质的基本和基本状态之一,但由于与高密度相关的困难导致多体相关性和缺乏远距离顺序,因此其物理理解远远落后于其他状态,例如气体和固态。液体科学中的重大开放问题包括玻璃过渡,结晶和水的异常。奥斯丁·安杰尔(Austen Angell)为这些问题做出了巨大贡献,并提出了许多基本重要性的新概念。在本文中,我们回顾了这些概念如何影响我们在液体物理学上的工作,重点关注液体结构有序在玻璃过渡,结晶和水异常中的作用。
The liquid state is one of the fundamental and essential states of matter, but its physical understanding is far behind the other states, such as the gas and solid states, due to the difficulties associated with the high density causing many-body correlations and the lack of long-range order. Significant open problems in liquid science include glass transition, crystallization, and water's anomalies. Austen Angell has contributed tremendously to these problems and proposed many new concepts of fundamental importance. In this article, we review how these concepts have influenced our work on liquid physics, focusing on the roles of liquid structural ordering in glass transition, crystallization, and water's anomalies.