论文标题

关键激子特性的直接测量:波函数的能量,动力学和空间分布

Direct measurement of key exciton properties: energy, dynamics and spatial distribution of the wave function

论文作者

Dong, Shuo, Puppin, Michele, Pincelli, Tommaso, Beaulieu, Samuel, Christiansen, Dominik, Hubener, Hannes, Nicholson, Christopher W., Xian, R. Patrick, Dendzik, Maciej, Deng, Yunpei, Windsor, Yoav William, Selig, Malte, Malic, Ermin, Rubio, Angel, Knorr, Andreas, Wolf, Martin, Rettig, Laurenz, Ernstorfer, Ralph

论文摘要

激子结合的电子孔对是控制半导体光电特性的基本激发。尽管已经对激子的光学特征进行了广泛的研究,但对激发功能函数本身的实验访问本身是难以捉摸的。使用多维光发射光谱,我们在分层半导体WSE $ _2 $中对激子的动量,能量和时间分辨的视角。通过调整激发波长,我们确定了明亮的激子形成的能量摩孔特征及其与常规单粒子激发态的差异。多维数据允许通过傅立叶变换来检索基本激子属性(例如结合能和激子晶格耦合),并通过傅立叶变换重建真实空间的激子分布函数。所有数量与微观计算都非常吻合。我们的方法提供了激子特性的完整表征,并适用于半导体材料,异质结构和设备中的明亮和深色激子。

Excitons, Coulomb-bound electron-hole pairs, are the fundamental excitations governing the optoelectronic properties of semiconductors. While optical signatures of excitons have been studied extensively, experimental access to the excitonic wave function itself has been elusive. Using multidimensional photoemission spectroscopy, we present a momentum-, energy- and time-resolved perspective on excitons in the layered semiconductor WSe$_2$. By tuning the excitation wavelength, we determine the energy-momentum signature of bright exciton formation and its difference from conventional single-particle excited states. The multidimensional data allows to retrieve fundamental exciton properties like the binding energy and the exciton-lattice coupling and to reconstruct the real-space excitonic distribution function via Fourier transform. All quantities are in excellent agreement with microscopic calculations. Our approach provides a full characterization of the exciton properties and is applicable to bright and dark excitons in semiconducting materials, heterostructures and devices.

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