论文标题
巡回电子密度波的语音辅助形成
Phonon-assisted formation of an itinerant electronic density wave
论文作者
论文摘要
电子不稳定性驱动凝结物质中的订购过渡。尽管对有序状态的微观理解取得了许多进步,但一个更细微和深刻的问题通常仍未得到解答:集体激发如何影响电子秩序形成?在这里,我们通过实验表明,声子会影响飞秒激光脉冲SDW猝灭后的自旋密度波(SDW)形成。在薄膜中,对温度依赖性的SDW周期进行了量化,从而使我们能够精确地跟踪SDW的不平衡形成路径。通过利用其持续的耦合到晶格,我们通过瞬态晶格失真探测了SDW,该速率通过飞秒X射线衍射测量。我们发现,在完全淬火后的500个飞秒之内,SDW形成低温时期,直接绕过具有高温周期的热状态。我们认为,由淬灭启动的动量匹配的声子通过顺序参数的动态固定来改变SDW的编队路径。
Electronic instabilities drive ordering transitions in condensed matter. Despite many advances in the microscopic understanding of the ordered states, a more nuanced and profound question often remains unanswered: how do the collective excitations influence the electronic order formation? Here, we experimentally show that a phonon affects the spin density wave (SDW) formation after an SDW-quench by femtosecond laser pulses. In a thin film, the temperature-dependent SDW period is quantized, allowing us to track the out-of-equilibrium formation path of the SDW precisely. By exploiting its persistent coupling to the lattice, we probe the SDW through the transient lattice distortion, measured by femtosecond X-ray diffraction. We find that within 500 femtoseconds after a complete quench, the SDW forms with the low-temperature period, directly bypassing a thermal state with the high-temperature period. We argue that a momentum-matched phonon launched by the quench changes the formation path of the SDW through the dynamic pinning of the order parameter.