论文标题

巡回电子密度波的语音辅助形成

Phonon-assisted formation of an itinerant electronic density wave

论文作者

Li, Jiaruo, Gorobtsov, Oleg Yu., Patel, Sheena K. K., Hua, Nelson, Gregory, Benjamin, Shabalin, Anatoly G., Hrkac, Stjepan, Wingert, James, Cela, Devin, Glownia, James M., Chollet, Matthieu, Zhu, Diling, Medapalli, Rajasekhar, Fullerton, Eric E., Shpyrko, Oleg G., Singer, Andrej

论文摘要

电子不稳定性驱动凝结物质中的订购过渡。尽管对有序状态的微观理解取得了许多进步,但一个更细微和深刻的问题通常仍未得到解答:集体激发如何影响电子秩序形成?在这里,我们通过实验表明,声子会影响飞秒激光脉冲SDW猝灭后的自旋密度波(SDW)形成。在薄膜中,对温度依赖性的SDW周期进行了量化,从而使我们能够精确地跟踪SDW的不平衡形成路径。通过利用其持续的耦合到晶格,我们通过瞬态晶格失真探测了SDW,该速率通过飞秒X射线衍射测量。我们发现,在完全淬火后的500个飞秒之内,SDW形成低温时期,直接绕过具有高温周期的热状态。我们认为,由淬灭启动的动量匹配的声子通过顺序参数的动态固定来改变SDW的编队路径。

Electronic instabilities drive ordering transitions in condensed matter. Despite many advances in the microscopic understanding of the ordered states, a more nuanced and profound question often remains unanswered: how do the collective excitations influence the electronic order formation? Here, we experimentally show that a phonon affects the spin density wave (SDW) formation after an SDW-quench by femtosecond laser pulses. In a thin film, the temperature-dependent SDW period is quantized, allowing us to track the out-of-equilibrium formation path of the SDW precisely. By exploiting its persistent coupling to the lattice, we probe the SDW through the transient lattice distortion, measured by femtosecond X-ray diffraction. We find that within 500 femtoseconds after a complete quench, the SDW forms with the low-temperature period, directly bypassing a thermal state with the high-temperature period. We argue that a momentum-matched phonon launched by the quench changes the formation path of the SDW through the dynamic pinning of the order parameter.

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