论文标题

通过单光束吸收光谱法解决非均匀温度分布。第二部分:宽带光谱实施

Resolving nonuniform temperature distributions with single-beam absorption spectroscopy. Part II: Implementation from broadband spectra

论文作者

Malarich, Nathan, Rieker, Greg

论文摘要

过去的几项研究描述了如何使用吸收光谱来通过测量对许多分子吸收过渡的温度的独特的非线性反应并进行反转来确定沿光路的空间温度变化。新的激光吸收光谱技术非常适合这种不均匀度测量,但是当前的分析方法仅使用孤立的特征,而不是完整的宽带光谱测量。在这项工作中,我们开发了一种被限制的光谱拟合技术,称为e“ - 固定,以适合不一致的环境引起的吸收光谱。我们通过使用双频率梳子激光测量来解决管炉中的对流电池来证明这种方法。每个测量高度处的恢复温度分布与现有的自然对流模型一致。最后,我们表明,对于具有噪声和吸收模型误差的实际测量值,增加带宽,测量的吸收过渡的数量可以提高温度分布精度。我们将拟合代码公开用于任何宽带吸收测量值。

Several past studies have described how absorption spectroscopy can be used to determine spatial temperature variations along the optical path by measuring the unique, nonlinear response to temperature of many molecular absorption transitions and performing an inversion. New laser absorption spectroscopy techniques are well-suited to this nonuniformity measurement, yet present analysis approaches use only isolated features rather than a full broadband spectral measurement. In this work, we develop a constrained spectral fitting technique called E"-binning to fit an absorption spectrum arising from a nonuniform environment. The information extracted from E"-binning is then input to the inversion approach from the previous paper in this series (Malarich and Rieker, JQSRT 107455) to determine the temperature distribution. We demonstrate this approach by using dual frequency comb laser measurements to resolve convection cells in a tube furnace. The recovered temperature distributions at each measurement height agree with an existing natural convection model. Finally, we show that for real-world measurements with noise and absorption model error, increasing the bandwidth and the number of measured absorption transitions may improve the temperature distribution precision. We make the fitting code publicly available for use with any broadband absorption measurement.

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