论文标题

二元氧化物纳米酰胺的结构演化,并通过退火及其对室温内部摩擦的影响

Structural evolution of binary oxide nanolaminates with annealing and its impact on room-temperature internal friction

论文作者

Yang, Le, Fazio, Mariana, Vajente, Gabriele, Ananyeva, Alena, Billingsley, GariLynn, Markosyan, Ashot, Bassiri, Riccardo, Fejer, Martin M., Menoni, Carmen S.

论文摘要

氧化物薄膜中的内部摩擦对超高技能对重力波探测器的灵敏度和稳定性的关键限制。寻求掺杂或创建纳米胺等策略,以引入减少内部摩擦的结构修饰。这项工作描述了对形态变化SiO2/TA2O5和TIO2/TA2O5纳米胺的研究,并随着退火及其对室温内部摩擦的影响。证明热处理导致两种纳米胺的内部摩擦减少,但通过不同的途径。在退火后层保持完整的SIO2/TA2O5纳米氨酸酯中,内部摩擦的总减少遵循组成的SIO2和TA2O5层的减少。取而代之的是,通过在TIO2/TA2O5纳米氨酸酯的界面退火而引发的交叉扩散和混合相的形成决定了内部摩擦的更明显的降低至〜2.6 * 10-4,其值低于任何其他具有相似阳离子浓度的TA2O5混合物。

Internal friction in oxide thin films imposes a critical limitation to the sensitivity and stability of ultra-high finesse optical cavities for gravitational wave detectors. Strategies like doping or creating nanolaminates are sought to introduce structural modifications that reduce internal friction. This work describes an investigation of the morphological changes SiO2/Ta2O5 and TiO2/Ta2O5 nanolaminates undergo with annealing and their impact on room temperature internal friction. It is demonstrated that thermal treatment results in a reduction of internal friction in both nanolaminates, but through different pathways. In the SiO2/Ta2O5 nanolaminate, which layers remain intact after annealing, the total reduction in internal friction follows the reduction in the composing SiO2 and Ta2O5 layers. Instead, interdiffusion initiated by annealing at the interface of the TiO2/Ta2O5 nanolaminate and the formation of a mixed phase dictate a more significant reduction in internal friction to ~ 2.6 * 10-4, a value lower than any other Ta2O5 mixture coating with similar cation concentration.

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