论文标题

观察两倍退化四倍的Weyl System Baptge中手性波函数

Observation of a Chiral Wave Function in Twofold Degenerate Quadruple Weyl System BaPtGe

论文作者

Li, Haoxiang, Zhang, Tiantian, Said, A., Fu, Y., Fabbris, G., Mazzone, D. G., Zhang, J., Lapano, J., Lee, H. N., Lei, H. C., Dean, M. P. M., Murakami, S., Miao, H.

论文摘要

量子材料中的拓扑状态由非平凡的拓扑不变式(例如Chern数字)定义,这些拓扑不变性是其批量波函数的特性。拓扑波函数的一个显着结果是边缘模式的出现,边缘模式(一种称为散装边缘对应的现象)产生了量化或手性的物理特性。虽然边缘模式被广泛地表示为非平凡拓扑的特征,但散装波函数如何显式表现出明确的拓扑特性仍未解决。在这里,使用高分辨率的非弹性X射线光谱(IXS)与第一原理计算相结合,我们报告了Baptge的散装声子频谱中手性波函数的实验性特征,我们向其显示以托管先前未发现的Twopert Twoford twoford twoford Quadenerate Quadenerate Quadruple Weyl Node。退化语音波函数的手性产生了一个非平凡的声子动力学结构因子S(Q,$ω$),沿高对称方向,与数值和模型计算非常吻合。我们的结果将IXs确定为揭示拓扑波函数的强大工具,在拓扑量子问题研究中提供了关键的缺失成分。

Topological states in quantum materials are defined by non-trivial topological invariants, such as the Chern number, which are properties of their bulk wave functions. A remarkable consequence of topological wave functions is the emergence of edge modes, a phenomenon known as bulk-edge correspondence, that gives rise to quantized or chiral physical properties. While edge modes are widely presented as signatures of non-trivial topology, how bulk wave functions can manifest explicitly topological properties remains unresolved. Here, using high-resolution inelastic x-ray spectroscopy (IXS) combined with first principles calculations, we report experimental signatures of chiral wave functions in the bulk phonon spectrum of BaPtGe, which we show to host a previously undiscovered twofold degenerate quadruple Weyl node. The chirality of the degenerate phononic wave function yields a non-trivial phonon dynamical structure factor, S(Q,$ω$), along high-symmetry directions, that is in excellent agreement with numerical and model calculations. Our results establish IXS as a powerful tool to uncover topological wave functions, providing a key missing ingredient in the study of topological quantum matter.

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