论文标题
观察两倍退化四倍的Weyl System Baptge中手性波函数
Observation of a Chiral Wave Function in Twofold Degenerate Quadruple Weyl System BaPtGe
论文作者
论文摘要
量子材料中的拓扑状态由非平凡的拓扑不变式(例如Chern数字)定义,这些拓扑不变性是其批量波函数的特性。拓扑波函数的一个显着结果是边缘模式的出现,边缘模式(一种称为散装边缘对应的现象)产生了量化或手性的物理特性。虽然边缘模式被广泛地表示为非平凡拓扑的特征,但散装波函数如何显式表现出明确的拓扑特性仍未解决。在这里,使用高分辨率的非弹性X射线光谱(IXS)与第一原理计算相结合,我们报告了Baptge的散装声子频谱中手性波函数的实验性特征,我们向其显示以托管先前未发现的Twopert Twoford twoford twoford Quadenerate Quadenerate Quadruple Weyl Node。退化语音波函数的手性产生了一个非平凡的声子动力学结构因子S(Q,$ω$),沿高对称方向,与数值和模型计算非常吻合。我们的结果将IXs确定为揭示拓扑波函数的强大工具,在拓扑量子问题研究中提供了关键的缺失成分。
Topological states in quantum materials are defined by non-trivial topological invariants, such as the Chern number, which are properties of their bulk wave functions. A remarkable consequence of topological wave functions is the emergence of edge modes, a phenomenon known as bulk-edge correspondence, that gives rise to quantized or chiral physical properties. While edge modes are widely presented as signatures of non-trivial topology, how bulk wave functions can manifest explicitly topological properties remains unresolved. Here, using high-resolution inelastic x-ray spectroscopy (IXS) combined with first principles calculations, we report experimental signatures of chiral wave functions in the bulk phonon spectrum of BaPtGe, which we show to host a previously undiscovered twofold degenerate quadruple Weyl node. The chirality of the degenerate phononic wave function yields a non-trivial phonon dynamical structure factor, S(Q,$ω$), along high-symmetry directions, that is in excellent agreement with numerical and model calculations. Our results establish IXS as a powerful tool to uncover topological wave functions, providing a key missing ingredient in the study of topological quantum matter.