论文标题

在2D量子自旋液体中成像旋子密度调制

Imaging spinon density modulations in a 2D quantum spin liquid

论文作者

Ruan, Wei, Chen, Yi, Tang, Shujie, Hwang, Jinwoong, Tsai, Hsin-Zon, Lee, Ryan, Wu, Meng, Ryu, Hyejin, Kahn, Salman, Liou, Franklin, Jia, Caihong, Aikawa, Andrew, Hwang, Choongyu, Wang, Feng, Choi, Yongseong, Louie, Steven G., Lee, Patrick A., Shen, Zhi-Xun, Mo, Sung-Kwan, Crommie, Michael F.

论文摘要

在某些条件下预测二维三角晶格抗铁磁铁,以表现出量子自旋液态基态,其低能量行为由Spinon Fermi表面描述。然而,由于其分数,无还清的性质,很难直接对产生的纺纱子进行成像。在这里,我们使用扫描隧道光谱来图像由单层1T键$ _2 $(二维Mott Mott Instrator)在单层Fermi表面不稳定性中产生的Spinon密度调制。我们首先证明了在单层1T键$ _2 $中排列在三角形晶格上的局部旋转,通过将其联系到金属1H-TASE $ _2 $ layer并测量近藤效应。随后的分离的单层1T键$ _2 $的光谱成像揭示了反映Spinon密度调制的Hubbard带能量的长波长调制。这允许对Spinon Fermi波形进行直接实验测量,这与2D量子自旋液体的理论预测很好地吻合。这些结果建立了单层1T键$ _2 $,作为研究新型二维量子旋转现象的新平台。

Two-dimensional triangular-lattice antiferromagnets are predicted under some conditions to exhibit a quantum spin liquid ground state whose low-energy behavior is described by a spinon Fermi surface. Directly imaging the resulting spinons, however, is difficult due to their fractional, chargeless nature. Here we use scanning tunneling spectroscopy to image spinon density modulations arising from a spinon Fermi surface instability in single-layer 1T-TaSe$_2$, a two-dimensional Mott insulator. We first demonstrate the existence of localized spins arranged on a triangular lattice in single-layer 1T-TaSe$_2$ by contacting it to a metallic 1H-TaSe$_2$ layer and measuring the Kondo effect. Subsequent spectroscopic imaging of isolated, single-layer 1T-TaSe$_2$ reveals long-wavelength modulations at Hubbard band energies that reflect spinon density modulations. This allows direct experimental measurement of the spinon Fermi wavevector, in good agreement with theoretical predictions for a 2D quantum spin liquid. These results establish single-layer 1T-TaSe$_2$ as a new platform for studying novel two-dimensional quantum-spin-liquid phenomena.

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