论文标题
通过高氧电子脉冲探测的结构动力学
Structural dynamics probed by high-coherence electron pulses
论文作者
论文摘要
超快测量技术为我们对固体和纳米结构的性质和功能的微观理解提供了重要的贡献。具有不断增长的空间和时间分辨率的原子尺度远景是通过基于X射线和电子短脉冲的方法提供的。时间分辨的电子衍射和显微镜是研究激发物质中非平衡结构动力学的最强大方法之一。在本文中,我们讨论了通过脉冲电子束的相干性的显着改善,超快电子成像的最新进展。具体而言,我们回顾了超快低能电子衍射(ULEED)的开发和首次应用,以研究表面上的结构动力学,并讨论了由激光触发的现场发射源促进的超快透射电子显微镜(UTEM)的新机会。这些和进一步的发展将使连贯的电子束成为超快纳米级成像的未来重要组成部分。
Ultrafast measurement technology provides essential contributions to our microscopic understanding of the properties and functions of solids and nanostructures. Atomic-scale vistas with ever-growing spatial and temporal resolution are offered by methods based on short pulses of x-rays and electrons. Time-resolved electron diffraction and microscopy are among the most powerful approaches to investigate non-equilibrium structural dynamics in excited matter. In this article, we discuss recent advances in ultrafast electron imaging enabled by significant improvements in the coherence of pulsed electron beams. Specifically, we review the development and first application of Ultrafast Low-Energy Electron Diffraction (ULEED) for the study of structural dynamics at surfaces, and discuss novel opportunities of Ultrafast Transmission Electron Microscopy (UTEM) facilitated by laser-triggered field emission sources. These and further developments will render coherent electron beams an essential component in the future of ultrafast nanoscale imaging.