论文标题
设备不对称和索特基屏障在2D光晶体管的螺旋依赖性光响应中的作用
The role of device asymmetries and Schottky barriers on the helicity-dependent photoresponse of 2D phototransistors
论文作者
论文摘要
圆形光电(CPC),即圆形光藻(CPGE)和光子阻力效应,最近在单层和多层过渡金属二甲藻元化(TMD)光晶体管中都报道了。但是,这些影响的出现的基本物理尚未完全理解。特别是,CPGE的出现与二维TMD的D3H晶体对称性不兼容,并且只有当电子状态的对称性通过诸如外部电场或机械应变之类的影响降低时,才有可能。 Schottky触点是基于TMD的晶体管几乎普遍存在的,可以提供高电场,从而导致设备中的对称性破坏。在这里,我们通过表征单层Mose2设备的螺旋依赖性光响应,均具有直接的金属Mose2 Schottky触点,以及在触点处具有H-BN隧道屏障,从而研究了这些Schottky接触对CPC的影响。我们发现,当设备中存在Schottky屏障时,允许对CPC的额外贡献,从而导致CPC在正常发病率下出现。
Circular photocurrents (CPC), namely circular photogalvanic (CPGE) and photon drag effects, have recently been reported both in monolayer and multilayer transition metal dichalcogenide (TMD) phototransistors. However, the underlying physics for the emergence of these effects are not yet fully understood. In particular, the emergence of CPGE is not compatible with the D3h crystal symmetry of two-dimensional TMDs, and should only be possible if the symmetry of the electronic states is reduced by influences such as an external electric field or mechanical strain. Schottky contacts, nearly ubiquitous in TMD-based transistors, can provide the high electric fields causing a symmetry breaking in the devices. Here, we investigate the effect of these Schottky contacts on the CPC by characterizing the helicity-dependent photoresponse of monolayer MoSe2 devices both with direct metal-MoSe2 Schottky contacts and with h-BN tunnel barriers at the contacts. We find that, when Schottky barriers are present in the device, additional contributions to CPC become allowed, resulting in emergence of CPC for illumination at normal incidence.