论文标题
在拥挤的环境中自行培养的Janus探测器的翻译和旋转动力学
Translational and rotational dynamics of a self-propelled Janus probe in crowded environments
论文作者
论文摘要
我们计算自行探针在拥挤的环境中的动态。拥挤是由粘弹性聚合物或非visCoalastic断开单体的存在引起的。我们的模拟表明,转化和旋转均方根位移,对于自我推广力的固定值具有独特的三步增长,而随着自我的影响,无论乌鸦的性质如何,随着自我推测而稳步增加。另一方面,在没有拥挤的人的情况下,Janus探测器的旋转动力学独立于自我推广力。在用粘性聚合物代替排斥聚合物时,Janus探针的翻译和旋转均方根位移显示出急剧下降。由于Janus粒子的不同面部与环境的相互作用不同,因此我们表明自我推测的方向也会影响其动力学。自行探针的长期翻译和旋转扩散率与固定的自我探测的比率(当针对人群的面积分数绘制时,都会经过最小值,而在没有众群体的情况下,较高的面积分数合并为其价值。这表明在人群中间区域的中间区域中,自行探针的转化和旋转动力学的脱钩。然而,对于被动探针,这种转移旋转的脱钩是不存在的。
We computationally investigate the dynamics of a self-propelled Janus probe in crowded environments. The crowding is caused by the presence of viscoelastic polymers or non-viscoelastic disconnected monomers. Our simulations show that the translational, as well as rotational mean square displacements, have a distinctive three-step growth for fixed values of self-propulsion force, and steadily increase with self-propulsion, irrespective of the nature of the crowder. On the other hand, in the absence of crowders, the rotational dynamics of the Janus probe is independent of self-propulsion force. On replacing the repulsive polymers with sticky ones, translational and rotational mean square displacements of the Janus probe show a sharp drop. Since different faces of a Janus particle interact differently with the environment, we show that the direction of self-propulsion also affects its dynamics. The ratio of long-time translational and rotational diffusivities of the self-propelled probe with a fixed self-propulsion, when plotted against the area fraction of the crowders, passes through a minima and at higher area fraction merges to its value in the absence of the crowder. This points towards the decoupling of translational and rotational dynamics of the self-propelled probe at intermediate area fraction of the crowders. However, such translational-rotational decoupling is absent for passive probes.