论文标题

FECR2TE4中Cr-Fe-Cr trimers的三维Ising Ferrimagnetism

Three-dimensional Ising Ferrimagnetism of Cr-Fe-Cr trimers in FeCr2Te4

论文作者

Liu, Yu, Koch, R. J., Hu, Zhixiang, Aryal, Niraj, Stavitski, Eli, Tong, Xiao, Attenkofer, Klaus, Bozin, E. S., Yin, Weiguo, Petrovic, C.

论文摘要

我们对三元基因化的单晶体中的磁性关键行为进行了全面研究,$ _2 $ _2 $ te $ _4 $在$ t_c $ $ $ \ sim $ 123 k下经历了铁磁过渡。关键指数$β= 0.30(1)$,$ t_c = 122.4(5)$ k,$γ,$γ= 1.22(1)$,$ t_c = 122.8(1)$ k,$δ= 4.24(2)$ at $ t_c $ $ \ $ \ sim $ \ sim $ 123 k表明,spins spins spins of spins of三维$ $ = 0.24 $ = 0.2555555555,和β5555,和$δ$ = 4.82)型号以及旋转之间有吸引力的远程相互作用,衰减为$ j(r)\大约r^{ - 4.88} $。我们的结果表明,FECR $ _2 $ te $ _4 $中的Ferrimagnetism是由于抗铁磁性耦合的CR-FE-CR Trimers中流动的铁磁性。

We carried out a comprehensive study of magnetic critical behavior in single crystals of ternary chalcogenide FeCr$_2$Te$_4$ that undergoes a ferrimagnetic transition below $T_c$ $\sim$ 123 K. Detailed critical behavior analysis and scaled magnetic entropy change indicate a second-order ferrimagentic transition. Critical exponents $β= 0.30(1)$ with $T_c = 122.4(5)$ K, $γ= 1.22(1)$ with $T_c = 122.8(1)$ K, and $δ= 4.24(2)$ at $T_c$ $\sim$ 123 K suggest that the spins approach three-dimensional Ising ($β$ = 0.325, $γ$ = 1.24, and $δ$ = 4.82) model coupled with the attractive long-range interactions between spins that decay as $J(r)\approx r^{-4.88}$. Our results suggest that the ferrimagnetism in FeCr$_2$Te$_4$ is due to itinerant ferromagnetism among the antiferromagnetically coupled Cr-Fe-Cr trimers.

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