论文标题

范德华晶体中的纳米级构造的Terahertz Polariton

Nanoscale-confined Terahertz Polaritons in a van der Waals Crystal

论文作者

de Oliveira, Thales V. A. G., Nörenberg, Tobias, Álvarez-Pérez, Gonzalo, Wehmeier, Lukas, Taboada-Gutiérrez, Javier, Obst, Maximilian, Hempel, Franz, Lee, Eduardo J. H., Klopf, John M., Errea, Ion, Nikitin, Alexey Y., Kehr, Susanne C., Alonso-Gonzaléz, Pablo, Eng, Lukas M.

论文摘要

电磁场的限制对于纳米光子技术至关重要,因为它允许增强光 - 物质的相互作用,从而在深层次波长尺度中实现轻度操纵。在Terahertz(THZ)光谱范围内,由于THZ辐射的波长相当长,因此通常使用特殊设计的金属结构(例如天线或纳米液)来实现辐射限制。在这种情况下,范德华(VDW)晶体中的声子Polaritons - 耦合到晶格振动的光已成为一种有前途的解决方案,可以控制超出衍射极限的光,因为它们具有极端的场限制和低光学损失。然而,到目前为止,在THZ频率处的纳米级构造声子极性子的实验证明仍然难以捉摸。在这里,我们通过使用散射型扫描近场光学显微镜(S-SNOM)以及自由电子激光(FEL)来提供它来提供它,以揭示VDW半导体$α-Moo_3 $的频率从8到12 THz的频率的一系列低损失极性激发。我们用i)可视化thz polaritons,ii)极端纳米级场限制(低于$λ_O/75 $)和iii)长极性寿命,下限为2 ps。

Electromagnetic field confinement is crucial for nanophotonic technologies, since it allows for enhancing light-matter interactions, thus enabling light manipulation in deep sub-wavelength scales. In the terahertz (THz) spectral range, radiation confinement is conventionally achieved with specially designed metallic structures - such as antennas or nanoslits - with large footprints due to the rather long wavelengths of THz radiation. In this context, phonon polaritons - light coupled to lattice vibrations - in van der Waals (vdW) crystals have emerged as a promising solution for controlling light beyond the diffraction limit, as they feature extreme field confinements and low optical losses. However, experimental demonstration of nanoscale-confined phonon polaritons at THz frequencies has so far remained elusive. Here, we provide it by employing scattering-type scanning near-field optical microscopy (s-SNOM) combined with a free-electron laser (FEL) to reveal a range of low-loss polaritonic excitations at frequencies from 8 to 12 THz in the vdW semiconductor $α-MoO_3$. We visualize THz polaritons with i) in-plane hyperbolic dispersion, ii) extreme nanoscale field confinement (below $λ_o/75$) and iii) long polariton lifetimes, with a lower limit of > 2 ps.

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