论文标题

阐明对2D周期物体的扫描隧道显微镜成像和空间频域中的晶体学平均值

Clarifying multiple-tip effects on Scanning Tunneling Microscopy imaging of 2D periodic objects and crystallographic averaging in the spatial frequency domain

论文作者

Straton, Jack C., Moeck, Peter, Moon Jr., Bill, Bilyeu, Taylor T.

论文摘要

晶体学图像处理(CIP)技术可以用于扫描探针显微镜(SPM)中,以收集因多个探针尖端信号所掩盖的信息。对于扫描隧道显微镜(STM),这可能非常重要,并且需要从二维周期性周期性的样品中的图像。与先前的方法相比,STM中多个提示的图像形成电流以更直接的方式得出。 P4MM Bloch表面波函数的电流的傅立叶光谱和一对Delta函数尖端揭示了各种形象的图像模糊的尖端分离依赖性。特别是我们的分析预测,量子干扰应以宏观尺度可见,以与篮子编织模式不同的频带的形式可见,纯经典模型将在同一周期性的双STM尖端分离中产生。引入并用于类似的尖端分离分析,并将其用于高度(0001)面向的热解石墨(技术称为HOPG)的基本特征的表面波函数。使用键合H_2尖端波函数具有显着的空间范围,而不是这对无限的无限dirac Delta功能尖端不会以任何可观察的方式影响这些结果。皮埃尔·库里(Pierre Curie)众所周知的对称原则来解释这一点。 STM图像中多个尖端效应的经典模拟可以理解为对其他类型的SPMS记录的图像中的多个尖端效应进行建模)。我们的分析阐明了为什么CIP和晶体学平均可以很好地消除从记录的2D周期性图像中从钝的SPM尖端(由多个小型TIPS组成)的效果,并概述了该图像处理技术对某些空间分离STM Minii Mini-Tips的局限性。

Crystallographic image processing (CIP) techniques may be utilized in scanning probe microscopy (SPM) to glean information that has been obscured by signals from multiple probe tips. This may be of particular importance for scanning tunneling microscopy (STM) and requires images from a sample that is periodic in two dimensions. The image-forming current for multiple tips in STM is derived in a more straightforward manner than prior approaches. The Fourier spectrum of the current for p4mm Bloch surface wave functions and a pair of delta function tips reveals the tip-separation dependence of various types of image obscurations. In particular our analyses predict that quantum interference should be visible on a macroscopic scale in the form of bands quite distinct from the basket-weave patterns a purely classical model would create at the same periodic double STM tip separations. A surface wave function that models the essential character of highly (0001) oriented pyrolytic graphite (technically known as HOPG) is introduced and used for a similar tip-separation analysis. Using a bonding H_2 tip wave function with significant spatial extent instead of this pair of infinitesimal Dirac delta function tips does not affect these outcomes in any observable way. This is explained by Pierre Curie's well known symmetry principle. Classical simulations of multiple tip effects in STM images may be understood as modeling multiple tip effects in images that were recorded with other types of SPMs). Our analysis clarifies why CIP and crystallographic averaging work well in removing the effects of a blunt SPM tip (that consist of multiple mini-tips) from the recorded 2D periodic images and also outlines the limitations of this image processing techniques for certain spatial separations of STM mini-tips.

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