论文标题
宽带全息辅助相干成像 - 朝着纳米级的Attosecond成像
Broadband holography-assisted coherent imaging -- towards attosecond imaging at the nanoscale
论文作者
论文摘要
近年来,纳米级相干成像已成为一种必不可少的成像方式,从而超过了经典成像光学的分辨率限制。同时,Attosond Science经历了巨大的进步,并揭示了原子,分子和复杂材料中的超快动态。将泵 - 探针实验与纳米空间分辨率的Attsond时间分辨率相结合,将允许在最小的时空尺度上研究超快动力学,但尚未得到证明。不幸的是,巨大的脉冲脉冲通常会阻碍高分辨率相干成像。在这里,我们提出了一种强大的全息增强相干成像方法,该方法允许将高质量和高空间分辨率相干成像与大光谱带宽相结合。通过在高谐波源上实施我们的方法,我们首次证明了34 nm(2.5λ)的空间分辨率与光谱带宽结合,支持傅立叶有限脉冲持续时间仅为380。该方法具有单发,还可以从测得的衍射模式中检索光谱,因此可以免疫射击波动。这为纳米级动力学的超快视图铺平了道路,例如超快电荷传输或超快自旋电流与PETAHERTZ电子和未来数据存储相关。
In recent years nanoscale coherent imaging has emerged as an indispensable imaging modality allowing to surpass the resolution limit given by classical imaging optics. At the same time, attosecond science has experienced enormous progress and has revealed the ultrafast dynamics in atoms, molecules, and complex materials. Combining attosecond temporal resolution of pump-probe experiments with nanometer spatial resolution would allow studying ultrafast dynamics on the smallest spatio-temporal scales but has not been demonstrated yet. Unfortunately, the large bandwidth of attosecond pulses usually hinders high-resolution coherent imaging. Here we present a robust holography-enhanced coherent imaging method, which allows combining high quality and high spatial resolution coherent imaging with a large spectral bandwidth. By implementing our method at a high harmonic source we demonstrate, for the first time, a spatial resolution of 34 nm (2.5 λ) in combination with a spectral bandwidth supporting a Fourier limited pulse duration of only 380 as. The method is single-shot capable, additionally retrieves the spectrum from the measured diffraction pattern, and is thus immune against shot-to-shot fluctuations. This paves the way for an ultrafast view on nanoscale dynamics e.g. ultrafast charge transfer or ultrafast spin currents being relevant for Petahertz electronics and future data storage.