论文标题

软固体表面的粘弹性和毛弹性松弛

Viscoelastic and poroelastic relaxations of soft solid surfaces

论文作者

Xu, Qin, Wilen, Lawrence A., Jensen, Katharine E., Style, Robert W., Dufresne, Eric R.

论文摘要

了解软固体的表面力学,例如软聚合物凝胶,在许多工程过程中至关重要,例如动态润湿和粘合性衰竭。在这些情况下,毛细管和弹性力的组合驱动了运动,通过耗散机制来平衡运动,以确定速率。尽管长期以来一直认为剪切流变学(即粘弹性)占主导地位,但最近的作品表明,压缩性效应(即毛弹性)可以在肿胀的网络中扮演角色。我们使用快速的干涉成像来量化由于移位的接触线而引起的表面变形的松弛。通过系统地测量不同时间和长度尺度的轮廓,我们从实验中观察到从粘弹性到毛弹性表面弛豫的交叉。

Understanding surface mechanics of soft solids, such as soft polymeric gels, is crucial in many engineering processes, such as dynamic wetting and adhesive failure. In these situations, a combination of capillary and elastic forces drives the motion, which is balanced by dissipative mechanisms to determine the rate. While shear rheology (i.e. viscoelasticity) has long been assumed to dominate the dissipation, recent works have suggested that compressibility effects (i.e. poroelasticity) could play roles in swollen networks. We use fast interferometric imaging to quantify the relaxation of surface deformations due to a displaced contact line. By systematically measuring the profiles at different time and length scales, we experimentally observe a crossover from viscoelastic to poroelastic surface relaxations.

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