论文标题

手性多胎半金属中的圆形光藻类作用的Ab-Initio研究

An ab-initio study of circular photogalvanic effect in chiral multifold semimetals

论文作者

Le, Congcong, Zhang, Yang, Felser, Claudia, Sun, Yan

论文摘要

到目前为止,圆形光藻(CPGE)是Weyl半含量中唯一可能的量化信号。随着反转和镜子对称性破裂,具有相反手势的带状结构中的Weyl和多fermions可以保持不同的能量并产生净拓扑电荷。这种净拓扑电荷可以在圆形极化诱导的注入电流中作为量化信号表示。根据当前的理论理解,RHSI及其对应物被认为是对量化CPGE进行实验观察的最有前途的候选人。但是,迄今为止,未在实验上观察到实际量化信号。由于量化CPGE的所有先前的理论研究都是基于有效模型但不是逼真的,因此它应该失去一些影响量化信号的关键细节。当前的状态动机我们为CPGE进行了现实的AB-Initio研究。我们的结果表明,量化值很容易被相关带相关的光学转换干扰,并且通过掺杂对化学电位进行微调对于观察量化的CPGE至关重​​要。这项工作基于逼真的电子带结构对量化的CPGE进行了第一个AB-Initio分析,并提供了解决给定材料当前问题的有效方法。

So far, the circular photogalvanic effect (CPGE) is the only possible quantized signal in Weyl semimetals. With inversion and mirror symmetries broken, Weyl and multifold fermions in band structures with opposite chiralities can stay at different energies and generate a net topological charge. Such kind of net topological charge can present as a quantized signal in the circular polarized light induced injection current. According to current theoretical understanding, RhSi and its counterparts are believed to be the most promising candidate for the experimental observation of the quantized CPGE. However, the real quantized signal was not experimentally observed to date. Since all the previous theoretical studies for the quantized CPGE were based on effective model but not realistic band structures, it should lose some crucial details that influence the quantized signal. The current status motives us to perform a realistic ab-initio study for the CPGE. Our result shows that the quantized value is very easy to be interfered by trivial bands related optic transitions, and an fine tuning of the chemical potential by doping is essential for the observation of quantized CPGE. This work performs the first ab-initio analysis for the quantized CPGE based on realistic electronic band structure and provides an effective way to solve the current problem for given materials.

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