论文标题
扭曲双层石墨烯的光学和等离子特性:层间隧道不对称和地面电荷不均匀性的影响
Optical and plasmonic properties of twisted bilayer graphene: Impact of interlayer tunneling asymmetry and ground-state charge inhomogeneity
论文作者
论文摘要
我们介绍了局部光学电导率,等离子体光谱和扭曲双层石墨烯(TBG)在不同填充因子和扭转角$θ$下的局部光学电导率和热电学性质的理论研究。我们的计算基于从连续模型获得的电子带结构,该模型具有两个可调参数,即$ u_0 $和$ u_1 $,该参数分别参数分别为sublattice Intratice Intratice Interlayer和sublattice Inter-Sublattice Inter-Layer Inter-Layer Inter-Layer隧道隧道率。在本文中,我们关注两个关键方面:i)我们研究结果对$ u_0 $的值的依赖性,探索整个范围$ 0 \ leq u_0 \ leq u_1 $; ii)我们考虑了由TBG中存在的固有电荷密度不均匀性产生的效果,通过计算自一致的Hartree近似中的带状结构。在零填充因子(即,在电荷中立性点,光导率都对$ u_0 $和扭转角的值非常敏感,而电荷不均匀性仅带来适度的校正。另一方面,远离零填充,静态筛选主导着,并且光导率显着受电荷不均匀性的影响,这是对其内带对其内贡献的最大效果。这些发现也由等离子光谱反映。我们将结果与文献中的现有结果进行比较,其中效果i)和ii)尚未系统地研究。作为我们计算的天然副产品,我们获得了Drude重量和塞贝克系数。前者显示出源于不均匀地面电荷分布的增强的颗粒孔不对称性。与单层石墨烯相比,即使在低温下($ \ rm k} $),后者即使在低温下($ \ rm k} $)也显示出广泛的标志变化功能。
We present a theoretical study of the local optical conductivity, plasmon spectra, and thermoelectric properties of twisted bilayer graphene (TBG) at different filling factors and twist angles $θ$. Our calculations are based on the electronic band structures obtained from a continuum model that has two tunable parameters, $u_0$ and $u_1$, which parametrize the intra-sublattice inter-layer and inter-sublattice inter-layer tunneling rate, respectively. In this Article we focus on two key aspects: i) we study the dependence of our results on the value of $u_0$, exploring the whole range $0\leq u_0\leq u_1$; ii) we take into account effects arising from the intrinsic charge density inhomogeneity present in TBG, by calculating the band structures within the self-consistent Hartree approximation. At zero filling factor, i.e. at the charge neutrality point, the optical conductivity is quite sensitive to the value of $u_0$ and twist angle, whereas the charge inhomogeneity brings about only modest corrections. On the other hand, away from zero filling, static screening dominates and the optical conductivity is appreciably affected by the charge inhomogeneity, the largest effects being seen on the intra-band contribution to it. These findings are also reflected by the plasmonic spectra. We compare our results with existing ones in the literature, where effects i) and ii) above have not been studied systematically. As natural byproducts of our calculations, we obtain the Drude weight and Seebeck coefficient. The former displays an enhanced particle-hole asymmetry stemming from the inhomogeneous ground-state charge distribution. The latter is shown to display a broad sign-changing feature even at low temperatures ($\approx 5~{\rm K}$) due to the reduced slope of the bands, as compared to those of single-layer graphene.