论文标题

固体中的强场电子动力学

Strong-Field Electron Dynamics in Solids

论文作者

Ishikawa, Kenichi L., Shinohara, Yasushi, Sato, Takeshi, Otobe, Tomohito

论文摘要

固态材料最近已成为强场物理学和ATTOSOND科学的新阶段。超时强烈激光脉冲驱动的电子动力学的机制正在深入讨论。在这里,我们从理论上讨论石墨烯和晶介质和半导体中的动量空间强场电子动力学。首先,在石墨烯的无质量狄拉克费米和紧密结合模型中,我们严格地得出了内的位移和带间跃迁,这构成了理解固态强场物理学(包括高谐波生成(HHG))的基础。然后,基于一维模型晶体的时间依赖性schrödinger方程,我们引入了一个简单的,多型,动量空间的三步模型,该模型结合了内部的位移,频带间隧道和与价带孔的重新组合。我们还分析了模型如何通过电子孔相互作用修饰。最后,研究了实际的三维材料。我们提出了一种时间依赖性的密度 - 矩阵方法,其HHG的结果与实验测量结果进行了比较。此外,我们使用实时依赖于时间依赖的密度功能理论来描述飞秒时间分辨率的动力学Franz-keldysh效应,即在激光场下的介电函数的时间依赖性调制。

Solid-state materials have recently emerged as a new stage of strong-field physics and attosecond science. The mechanism of the electron dynamics driven by an ultrashort intense laser pulse is under intensive discussion. Here we theoretically discuss momentum-space strong-field electron dynamics in graphene and crystalline dielectrics and semiconductors. First, within massless Dirac fermion and tight-binding models for graphene, we rigorously derive intraband displacement and interband transition, which form the basis for understanding solid-state strong-field physics including high-harmonic generation (HHG). Then, based on the time-dependent Schrödinger equation for a one-dimensional model crystal, we introduce a simple, multiband, momentum-space three-step model that incorporates intraband displacement, interband tunneling, and recombination with a valence band hole. We also analyze how the model is modified by electron-hole interaction. Finally, actual three-dimensional materials are investigated. We present a time-dependent density-matrix method whose results for HHG are compared with experimental measurement results. Moreover, we describe the dynamical Franz-Keldysh effect in femtosecond time resolution, i.e., the time-dependent modulation of a dielectric function under an intense laser field, using a real-time time-dependent density functional theory.

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