论文标题

铁磁Eutio $ _ {3} $(001)的(001)表面(001)表面的二维电子气

A two-dimensional electron gas at the (001) surface of ferromagnetic EuTiO$_{3}$(001)

论文作者

Di Capua, R., Verma, M., Radovic, M., Plumb, N. C., Dil, J. H., Ristic, Z., Guedes, E. B., De Luca, G. M., Preziosi, D., Wang, Z., Weber, A. P., Pentcheva, R., Salluzzo, M.

论文摘要

氧化物准二维电子气体(Q2DEG)的研究一直是发现新颖的,有时是意外现象的操场,例如报告的磁性在表面上的磁性以及Laalo $ _ {3} $ {3} $和SRTIO $ _ {3} $ _ {3} $非磁性材料之间的界面。但是,该系统中的磁性很弱,并且有没有内在起源的证据。在这里,通过使用原位高分辨率角度分辨光发射,我们证明了批量的srtio $ _ {3} $的铁磁Eutio $ _ {3} $,在其(001)表面托管Q2DEG。这是通过在各种构型中存在氧气分裂的情况下用哈伯u术语的密度功能理论计算来证实的,所有这些都会导致与欧盟4F磁矩的铁磁顺序相关的自旋偏振Q2DEG。结果表明Eutio $ _ {3} $(001)是氧化物Q2DEGS的新材料平台,其特征是反转和时间反向对称性。

Studies on oxide quasi-two dimensional electron gas (q2DEG) have been a playground for the discovery of novel and sometimes unexpected phenomena, like the reported magnetism at the surface and at the interface between LaAlO$_{3}$ and SrTiO$_{3}$ non-magnetic materials. However, magnetism in this system is weak and there are evidences of a not intrinsic origin. Here, by using in-situ high-resolution angle resolved photoemission we demonstrate that ferromagnetic EuTiO$_{3}$, the magnetic counterpart of SrTiO$_{3}$ in the bulk, hosts a q2DEG at its (001) surface. This is confirmed by density functional theory calculations with Hubbard U terms in the presence of oxygen divacancies in various configurations, all of them leading to a spin-polarized q2DEG related to the ferromagnetic order of Eu-4f magnetic moments. The results suggest EuTiO$_{3}$(001) as a new material platform for oxide q2DEGs, characterized by broken inversion and time reversal symmetries.

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