论文标题

超快动态LIFSHITZ过渡

Ultrafast Dynamical Lifshitz Transition

论文作者

Beaulieu, Samuel, Dong, Shuo, Tancogne-Dejean, Nicolas, Dendzik, Maciej, Pincelli, Tommaso, Maklar, Julian, Xian, R. Patrick, Sentef, Michael A., Wolf, Martin, Rubio, Angel, Rettig, Laurenz, Ernstorfer, Ralph

论文摘要

费米表面是我们对金属的理解和密切相关的多体系统的核心。费米表面拓扑的突然变化,也称为Lifshitz过渡,可能导致引人入胜的现象的出现,例如巨大的磁磁性和超导性。尽管通过宏观参数(例如应变,掺杂,压力和温度)的平衡调谐,已经证明了LIFSHITZ的转变,但未通过实验证明,非平衡的动力学途径,但尚未证明非平衡的动力学途径。将时间分辨的多维光发射光谱与最先进的TDDFT+$ U $模拟相结合,我们引入了一种新颖的方案,用于在相关类型的II型Weyl Semimetal T $ \ Mathrm {_ {_ {d} $ - Mote-Mote $ $ _} $ _ {2}中驱动超富含LIFSHITZ的过渡。我们证明,这种非平衡拓扑电子过渡在有效电子相关的动态修饰中发现了其显微镜起源。这些结果揭示了一种新型的超快方案,该方案用于控制相关量子材料中的费米表面拓扑。

Fermi surface is at the heart of our understanding of metals and strongly correlated many-body systems. An abrupt change in the Fermi surface topology, also called Lifshitz transition, can lead to the emergence of fascinating phenomena like colossal magnetoresistance and superconductivity. While Lifshitz transitions have been demonstrated for a broad range of materials by equilibrium tuning of macroscopic parameters such as strain, doping, pressure and temperature, a non-equilibrium dynamical route toward ultrafast modification of the Fermi surface topology has not been experimentally demonstrated. Combining time-resolved multidimensional photoemission spectroscopy with state-of-the-art TDDFT+$U$ simulations, we introduce a novel scheme for driving an ultrafast Lifshitz transition in the correlated type-II Weyl semimetal T$\mathrm{_{d}}$-MoTe$_{2}$. We demonstrate that this non-equilibrium topological electronic transition finds its microscopic origin in the dynamical modification of the effective electronic correlations. These results shed light on a novel ultrafast scheme for controlling the Fermi surface topology in correlated quantum materials.

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