论文标题
低能量干扰结构,具有时间分辨率
Low-Energy Interference Structure with Attosecond Temporal Resolution
论文作者
论文摘要
准确地访问电子波包(EWP)的相位变化提供了前所未有的时空信息。在强场光电离实验中已广泛观察到接近零能的径向干扰模式。但是,这种干扰模式的基本物理图片仍在争论中。在这里,我们报告了对中红外激光场这种低能干扰结构(LIE)的实验和理论研究。我们阐明了由于软重新卷曲机制而产生的leis产生,以前发现该机制在产生明显的低能结构中起着关键作用。具体而言,在我们的实验中,在1/18激光循环时间范围内发射的直接和软回收EWP之间的干扰引起了LIE。此外,LEI的观察与激光波长和特定原子靶标无关。我们的结果开辟了一个有希望的新途径,用于检索通过attseent Time分辨率的原子和分子中EWP的结构和动力学。
Accessing precisely to the phase variation of electronic wave-packet (EWP) provides unprecedented spatiotemporal information of microworld. A radial interference pattern at near-zero energy has been widely observed in experiments of strong-field photoionization. However, the underlying physical picture of this interference pattern is still under debate. Here we report an experimental and theoretical investigation of this low-energy interference structure (LEIS) in mid-infrared laser fields. We clarify that the LEIS arises due to the soft-recollision mechanism, which was previously found to play a pivotal role in producing the pronounced low-energy structure. Specifically, the LEIS is induced by the interference between direct and soft-recollision EWPs launched within a 1/18 laser-cycle time scale in our experiments. Moreover, the observation of LEIS is independent of laser wavelength and specific atomic targets. Our result opens a promising new avenue for retrieving the structure and dynamics of EWPs in atoms and molecules with attosecond time resolution.